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- W4312141036 abstract "The development of transition metal-catalyzed β-C-H bond activation via highly-strained 4-membered metallacycles has been a formidable task. So far, only scarce examples have been reported to undergo β-C-H bond activation via 4-membered metallacycles, and all of them rely on precious metals. In contrast, earth-abundant and inexpensive 3d transition metal-catalyzed β-C-H bond activation via 4-membered metallacycles still remains an elusive challenge. Herein, we report a phosphine oxide-ligated Ni-Al bimetallic catalyst to activate secondary benzylic C(sp3)-H bonds of formamides via 4-membered nickelacycles, providing a series of α,β-unsaturated γ-lactams in up to 97% yield." @default.
- W4312141036 created "2023-01-04" @default.
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- W4312141036 date "2022-12-22" @default.
- W4312141036 modified "2023-10-17" @default.
- W4312141036 title "Ni-catalyzed benzylic β-C(sp3)–H bond activation of formamides" @default.
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- W4312141036 doi "https://doi.org/10.1038/s41467-022-35541-6" @default.
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