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• W4319459405 abstract "Application of femtosecond time-resolved transient absorption spectroscopy on all-trans and central-cis isomers of two exemplary carotenoids, lutein and spirilloxanthin, performed at room and cryogenic temperatures in the spectral range expanded toward UV revealed new spectroscopic transient features for the cis isomers. Notably, particularly for the central-cis spirilloxanthin, a very distinct additional transient absorption band is observed on the short wavelength side of the main excited-state absorption band of the S1 state, having the same temporal characteristics as the latter one. This band is absent in transient absorption spectra of all-trans isomers, suggesting it could be assigned to transient cis-peak. Overall, the results show that the transient counterpart of the spectral marker of cis-isomers of carotenoids, or the so-called cis-peak, is detectable in the excited-state absorption spectrum and could be attributed to electronic transition from the S1 state. This new transient spectral band could be very useful for spectroscopic experiments targeting the dynamics of carotenoid isomers and their severely distorted forms." @default.
• W4319459405 created "2023-02-09" @default.
• W4319459405 creator A5061217120 @default.
• W4319459405 date "2023-02-08" @default.
• W4319459405 modified "2023-10-16" @default.
• W4319459405 title "Transient “<i>cis</i>-Peak” Is Present in Excited-State Absorption of Central-<i>cis</i> Isomers of Carotenoids" @default.
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• W4319459405 doi "https://doi.org/10.1021/acs.jpclett.2c03855" @default.
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