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- W10010756 abstract "Heteropolyacids (HPA) with the Keggin structure, H3[PM12O40] (M = Mo, W), used as precursors for the oxidation of organic substrates in homogeneous or biphase systems are degraded in the presence of excess H2O2. This process has been studied by spectrometric methods (UV spectroscopy, Raman diffusion, …). Aqueous solutions of H3[PM12O40] treated with an excess of hydrogen peroxide (30 ≤ [H2O2]/[M] ≤ 355) lead to the peroxo species [M2O3(O2)4(H2O)2]2-, , and {PO4[MO(O2)2]4}3-, , which have been proposed previously and independently as active-oxygen-to-olefin transfer agents in homogeneous systems or under phase transfer reaction conditions. Other precursors with the Keggin moiety, H5[BW12O40] and H4[SiW12O40] or with the Dawson structure, H6[P2W18O62], have been considered in order to establish a relationship between the catalytic activity and the products formed in the HPA-H2O2 systems." @default.
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- W10010756 date "1991-01-01" @default.
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- W10010756 title "New insights into the catalytic activity of polyoxometalates for oxidation with hydrogen peroxide" @default.
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- W10010756 doi "https://doi.org/10.1016/s0167-2991(08)62872-4" @default.
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