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- W1008058157 abstract "A model bioethanol steam reforming reaction is performed in a thin composite Pd membrane reactor by using Ni/CeO2 catalyst. A 7.5 wt.% Ni/CeO2 catalyst was prepared by Solution Combustion Synthesis using urea as fuel. The obtained powder was characterized by X-ray diffraction (XRD), N2-physisorption, CO-chemisorption and temperature programmed reduction (TPR). A 8 μm thin Pd-layer deposited onto a porous Al2O3 support constitutes the membrane allocated in the membrane reactor module, where the catalyst is packed in the annulus. The H2 perm-selectivity of the composite membrane (expressed as H2/N2 ideal selectivity) is around 4700 at 400 °C, Δp = 0.5 bar and in fresh membrane conditions. The bioethanol reforming is carried out at 400 °C and the reaction pressure ranges from 2.0 to 3.0 bar as well as GHSV from 5000 to 15,000 h−1. The best performance of the membrane reactor is achieved at 400 °C, 3.0 bar and GHSV = 5000 h−1 where the ethanol conversion is around 98%, with more than 65% of hydrogen recovered in the permeate side. Furthermore, the influence of the byproducts present as impurities in the model bioethanol mixture on the membrane reactor performance is also evaluated." @default.
- W1008058157 created "2016-06-24" @default.
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- W1008058157 date "2016-01-01" @default.
- W1008058157 modified "2023-10-18" @default.
- W1008058157 title "The oncoming energy vector: Hydrogen produced in Pd-composite membrane reactor via bioethanol reforming over Ni/CeO 2 catalyst" @default.
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- W1008058157 doi "https://doi.org/10.1016/j.cattod.2015.04.046" @default.
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