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- W10336716 abstract "The dephasing signals of the 14N2 vibron in pure α-N2 [1] and in mixed crystals with 15N2 [1] or Ar, [2] were measured using time-resolved coherent anti-Stokes Raman scattering (TR-CARS). Our experimental results could be well fitted [1,2] starting from the ad-hoc assignement of the homogeneous and the inhomogeneous component in the frequency domain respectively as a Lorentzian and a Gaussian lineshape. However, recently we performed high-resolution spontaneous Raman scattering measurements using Fabry-Perot interferometry on a mixed crystal of α-(15N2)0.013(14N2)0.937Ar0.05 The small concentration of 15N2 molecules admixed in the crystal allows us to compare the excitonic line-shapes with these of localized vibrations, while it has only a minor effect [1] on the 14N2 vibron lineshape. As can be seen in Fig. 1, both the A g mode and the Tg mode of the k ≃ 0 vibron have asymmetrical lineshapes. This is in clear contrast to what was assumed for fitting our time domain measurements." @default.
- W10336716 created "2016-06-24" @default.
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- W10336716 date "1994-01-01" @default.
- W10336716 modified "2023-09-27" @default.
- W10336716 title "Restrictions to Homodyne Time-Resolved Techniques: Asymmetric Lineshapes of the Vibrons in α-Ar x (N2)1−x" @default.
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- W10336716 doi "https://doi.org/10.1007/978-3-642-85060-8_11" @default.
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