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- W103643924 abstract "Iron containing micro-and mesoporous substances were exposed to various treatments and changes in coordination and oxidation states of iron are analyysed. ZSM-5 (Si/Fe=200) and MCM-22 (Si/Fe=13.5) are applied as microporous hosts. Most of iron is stabilized in tetrahedral framework positions in the first structure, whereas profound rearrangements may proceed on iron with simultaneous redox processes in the second host. SBA-15 (Si/Fe=76) and MCM-41 (Si/Fe=50) were selected as mesoporous matrices. The partly amorphous feature of the pore walls is reflected in coordinations occupied by iron. Fe 3+ → Fe 2+ reversible redox transformations may proceed in large part of iron. Further, novel types of coordinations appear which cannot be detected in microporous hosts." @default.
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- W103643924 date "2005-01-01" @default.
- W103643924 modified "2023-10-16" @default.
- W103643924 title "Stabilization of iron in micro-and mesoporous ferrisilicates (MFI, MCM-22, SBA-15, and MCM-41) as detected by in situ mössbauer spectroscopy" @default.
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- W103643924 doi "https://doi.org/10.1016/s0167-2991(05)80407-0" @default.
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