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- W1098491843 abstract "Abstract In transient absorption (TA) spectra, the bleach features originating from state filling are overlapped by their energy-shifted derivatives, arising from excited state energy level shifts. This makes the direct extraction of carrier dynamics from a single-wavelength time-trace misleading. Fitting TA spectra in time, as Gaussian functions and their derivative-like shifted Gaussians, allows to individually extract the real dynamics of both photobleached transitions, and their energy shifts. In CdTe nanorods (NRs) we found a delayed heating of holes due to the release of the large excess energy in the electron relaxation process. The slow hole-trapping process is consistent with a high number of surface trap states in these model NRs. Our results show that only a correct disentanglement of bleaching and energy shift contributions provides a reliable framework to extract the underlying carrier relaxation dynamics, including trapping, non-radiative recombination, and eventually carrier multiplication." @default.
- W1098491843 created "2016-06-24" @default.
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- W1098491843 date "2016-06-01" @default.
- W1098491843 modified "2023-09-23" @default.
- W1098491843 title "Delayed electron relaxation in CdTe nanorods studied by spectral analysis of the ultrafast transient absorption" @default.
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- W1098491843 doi "https://doi.org/10.1016/j.chemphys.2015.08.002" @default.
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