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- W112192222 abstract "The probable dissolution mechanisms for UO/sub 2/ and spent fuel were studied based on accelerating oxidation and dissolutions in autoclave and electrochemical experiments. The dissolution of UO/sub 2/ is primarily due to oxidation of U/sup +4/ (solid) to U/sup +6/ (liquid). The U/sup +6/(liquid) is initially in dissolved uranyl ions, UO/sub 2//sup +2/, but subsequent hydrolysis reactions lead to the formation of solid uranyl hydrates (or related complex compounds) that deposit onto the surfaces of UO/sub 2/ and container walls as thin or thick coatings, depending on the temperature, pH, and time. Therefore, the dissolution rate of UO/sub 2/ cannot be simply determined from the uranium content of the solution. Moreover, the dissolution rate is not limited by the solubility of the uranyl ions. Electrochemical dissolution of spent fuel shows that the initial dissolution and leaching behavior is similar to that of UO/sub 2/ surfaces." @default.
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- W112192222 date "1980-01-01" @default.
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- W112192222 title "Dissolution mechanisms for UO/sub 2/ and spent fuel" @default.
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