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- W113149526 abstract "Reactions of COH2 mixtures have been studied on a series of PdSiO2 catalysts (2 wt% Pd) with and without a promoting additive. Mg and La compounds were used as promoters. It appeared that promoters (i) influence the activity of the catalysts and (ii) increase the selectivity for “oxygenates” and suppress the selectivity for CH4. The activity for methanol synthesis is linearly correlated with the amount of Pd extractable from the reduced and used catalysts as Pd-acetylacetonate. Since it is known that promoters also create a new type of ionic adsorption center for CO and NO adsorption, it is concluded that Pd “ions” are indeed the centers for activation of CO toward methanol whereas Pd metal supplies hydrogen atoms for hydrogenation." @default.
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- W113149526 date "1983-07-01" @default.
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- W113149526 title "On the selectivity of palladium catalysts in synthesis gas reactions" @default.
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- W113149526 doi "https://doi.org/10.1016/0021-9517(83)90114-8" @default.
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