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- W1131619385 abstract "The mechanistic studies for linear cross-dimerization between 2,3-dimethylbuta-1,3-diene and styrene by a Ru(0) complex, Ru(η6-naphthalene)(η4-1,5-COD) (1), are performed both by kinetic and computational studies. This reaction is basically zero-order to both of the diene and styrene concentrations and first-order to the catalyst concentration. The Hammett plot using p-substituted styrenes gives a linear relationship with a positive slope (ρ = +0.482). The deuterium isotope experiment clearly shows the present reaction being a formal 1,4-addition of a C–H bond in styrene to cisoid-1,3-diene. These kinetic studies show the reaction proceeding via oxidative coupling mechanism that is also supported by the DFT calculations." @default.
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- W1131619385 date "2015-11-01" @default.
- W1131619385 modified "2023-09-23" @default.
- W1131619385 title "Mechanistic insights into catalytic linear cross-dimerization between conjugated dienes and styrenes by a ruthenium(0) complex" @default.
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- W1131619385 doi "https://doi.org/10.1016/j.jorganchem.2015.08.022" @default.
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