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- W113400162 abstract "For some time now in our laboratory we have been using well-mixed, ''gradientless'' reactors to study the dynamics of gas-carbon reactions. In the past we have used a mechanically-stirred, Berty-type reactor to examine the kinetics of carbon dioxide and steam gasification of chars. More recently, we have been involved in investigating the behavior of ''active sites'' in certain carbonaceous chars. As a result of the requirements of this work, we were led to the development of a jet-stirred, ''gradientless'' reactor. The current paper describes the design, development and application of this reactor to char gasification studies. The research project for which the reactor was developed is concerned with the study of the nature and behavior of ''active sites'' in the gasification of chars produced from synthesized model compounds, primarily those of the phenol-formaldehyde family of resins. One of the tasks defined for this project was to conduct transient kinetic studies on the gasification of these model compound chars, for both unlabelled and /sup 13/C-labelled resins. Due to the requirements of the expense of the labelled resins we were led to a design that minimized the relatively large sample requirements of the existing autoclave reactor. Once the necessity for developing amore » new reactor was realized, it was decided to employ jet-mixing in order to avoid some of the potential complexities of mechanical mixing under the particular operating conditions dictated by the nature of the reaction system. 6 refs., 8 figs., 1 tab.« less" @default.
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- W113400162 date "1986-01-01" @default.
- W113400162 modified "2023-09-27" @default.
- W113400162 title "A jet-stirred reactor for transient studies of char gasification" @default.
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