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• W1163011906 abstract "An unprecedented N-heterocyclic carbene (NHC)-catalyzed annulation of enals to form 3,4-disubstituted cyclopentanones has been discovered. Aryl enals undergo dimerization in the presence of a single-electron oxidant to form C2 symmetric cyclopentanones. A cross-reaction has also been developed, allowing for the synthesis of differentially substituted cyclopentanones. Mechanistically, the reaction is thought to proceed through radical intermediates, further establishing the synthetic utility of this class of reactivity." @default.
• W1163011906 created "2016-06-24" @default.
• W1163011906 creator A5074994681 @default.
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• W1163011906 date "2015-08-10" @default.
• W1163011906 modified "2023-10-18" @default.
• W1163011906 title "Oxidatively Initiated NHC-Catalyzed Enantioselective Synthesis of 3,4-Disubstituted Cyclopentanones from Enals" @default.
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• W1163011906 doi "https://doi.org/10.1021/jacs.5b06390" @default.
• W1163011906 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/4986695" @default.
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