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- W1163142785 abstract "This work introduces a new strategy for visible/near-infrared (NIR) light responsive H2 production over TiO2 nanoparticles co-sensitized with zinc phthalocyanine derivative (Zn-tri-PcNc) and surface ligand-to-metal charge transfer (LMCT) complex, which is in situ formed on the TiO2 nanoparticles' surfaces by using ascorbic acid (AA). The in situ formed surface LMCT complex (AA-TiO2) exhibits obvious visible-light-responsive photoactivity (126.2 μmol/h) for H2 production with a high apparent quantum yield (AQY) of 16.1% at 420 nm monochromatic light irradiation. Moreover, the co-sensitized TiO2 nanoparticles (Zn-tri-PcNc-TiO2-AA) shows a much higher photoactivity (162.2 μmol/h) for H2 production than the surface LMCT complex, and broader spectral responsive region (400–800 nm) with a relatively high AQY value (0.97%) at 700 nm monochromatic light irradiation. The present result reveals a possible substitute for the conventional Ru(II)-bipyridyl complexes or organic dyes as sensitizer of semiconductors in the field of solar fuel conversion." @default.
- W1163142785 created "2016-06-24" @default.
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- W1163142785 date "2015-12-01" @default.
- W1163142785 modified "2023-10-17" @default.
- W1163142785 title "A new route for visible/near-infrared-light-driven H2 production over titania: Co-sensitization of surface charge transfer complex and zinc phthalocyanine" @default.
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- W1163142785 doi "https://doi.org/10.1016/j.jpowsour.2015.08.040" @default.
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