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- W1176292100 abstract "The study evaluates the capacity fade of commercial 3.25 Ah 18650-type cells with NCA cathodes and graphite anodes quantitatively for different temperatures and charging strategies. For standard constant current / constant voltage (CC-CV) charging, the aging rate for cells cycled at 0.5C is increased with decreasing temperature in the range of 25 °C to 0 °C. Interestingly, no accelerated aging is observed for CC-CV charging in the temperature range of 25 °C to 60 °C at 0.5C. The observed behavior indicates lithium deposition on anodes for temperatures up to ∼25 °C and is further investigated by reconstruction of anode and cathode from the commercial 18650-type cells into full cells with an additional lithium metal reference electrode. The reconstruction method is scrutinized regarding its validity. Measurements with the reconstructed cells at 25 °C reveal the quantitative dependency of the anode potential vs. Li/Li+ from the charge C-rate and cell voltage. This allows deriving charging strategies involving strictly positive anode potentials to avoid lithium deposition and preventing the corresponding capacity fade." @default.
- W1176292100 created "2016-06-24" @default.
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- W1176292100 date "2015-10-01" @default.
- W1176292100 modified "2023-10-18" @default.
- W1176292100 title "Optimization of Charging Strategy by Prevention of Lithium Deposition on Anodes in high-energy Lithium-ion Batteries – Electrochemical Experiments" @default.
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- W1176292100 doi "https://doi.org/10.1016/j.electacta.2015.08.056" @default.
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