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- W1211893603 startingPage "6521" @default.
- W1211893603 abstract "Inelastic neutron scattering from clusters of ${mathrm{Co}}^{2+}$ ions in cubic KZn${mathrm{F}}_{3}$ is reported. From measurements of the lowest pair mode at (1.676ifmmodepmelsetextpmfi{}0.008) THz, we find that the exchange between ${mathrm{Co}}^{2+}$ ions is surprisingly isotropic, with any bond anisotropy being less than 2.4%. An accurate value of the isotropic exchange parameter has been obtained [$J=(0.330ifmmodepmelsetextpmfi{}0.005)$ THz] free of the many-body effects that complicate the interpretation of exchange coupling in concentrated crystals. Neutron scattering was also observed from triplet and quartet states at (2.47ifmmodepmelsetextpmfi{}0.02) and (1.09ifmmodepmelsetextpmfi{}0.05) THz, respectively, and a higher-frequency pair state at 8.8 THz. The results are interpreted in terms of an elementary theory of cluster spectra for ions with nonzero angular momentum." @default.
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- W1211893603 date "1984-12-01" @default.
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- W1211893603 title "Excitations of isolated clusters ofCo2+magnetic ions in KZn0.92Co0.08F3" @default.
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- W1211893603 doi "https://doi.org/10.1103/physrevb.30.6521" @default.
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