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- W122220887 abstract "The structure of water attached to glass can affect the thermodynamics as well as the mechanism of the solution adsorption of flexible macromolecules, such as native proteins, capable of undergoing surface-induced conformational changes. Although both components of the glass/water adsorption system are quite common, even the modern literature has little, if any, information applicable to a quantitative characterization of the state of sorbed water. From a soda-lime type glass containing TiO 2 and BaO, particles were prepared measuring ≤1μ in the SEM. After exhaustive acid leaching and washings with water, the powder obtained had a B.E.T. specific surface area of 9.85 m 2 /g. Using this adsorbent, its heats of immersion into water, which did not vary with surface area, were measured at 25° and 37°C in a thermistori zed isothermal-jacketed microcalorimeter capable of resolving ±1 × 10 −50 C in 100 ml of liquid volume. The 0°, 25° and 37°C water vapor adsorption isotherms of the powder determined at relative pressures ≥5 × 10 −5 indicated no hysteresis and the absence of porosity. The vapor adsorption data have been analyzed according to the B.E.T. and the deBoer-Zwikker-Bradley methods. Consistent with the standard thermodynamic functions computed from the adsorption isotherms, the heat of immersion data indicate that, on this particular glass, inter-facial water becomes ordered to a depth of 8-10 monolayers and its state is about 5-6 e.u. below that of bulk water at identical temperatures." @default.
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- W122220887 date "1976-01-01" @default.
- W122220887 modified "2023-09-26" @default.
- W122220887 title "THE STATE OF WATER ADJACENT TO GLASS" @default.
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- W122220887 doi "https://doi.org/10.1016/b978-0-12-404503-3.50053-7" @default.
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