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• W1243823141 abstract "Nonlinear frequency conversion offers an effective way to expand the laser wavelength range based on birefringence phase matching (BPM) or quasi-phase-matching (QPM) techniques in nonlinear crystals. So far, efficient high-harmonic generation is enabled only via multiple cascaded crystals because of the extreme difficulty to simultaneously satisfy BPM or QPM for multiple nonlinear up-conversion processes within a single crystal. Here we report the design and fabrication of a chirped periodic poled lithium niobate (CPPLN) nonlinear crystal that offers controllable multiple QPM bands to support 2nd--8th harmonic generation (HG) simultaneously. Upon illumination of a mid-IR femtosecond pulse laser, we observe the generation of an ultrabroadband visible white light beam corresponding to 5th--8th HG with a record high conversion efficiency of 18%, which is high compared to conventional supercontinuum generation, especially in the HG parts. Our CPPLN scheme opens up a new avenue to explore and engineer novel nonlinear optical interactions in solid state materials for application in ultrafast lasers and broadband laser sources." @default.
• W1243823141 created "2016-06-24" @default.
• W1243823141 creator A5013194814 @default.
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• W1243823141 date "2015-08-20" @default.
• W1243823141 modified "2023-09-28" @default.
• W1243823141 title "High-Efficiency Broadband High-Harmonic Generation from a Single Quasi-Phase-Matching Nonlinear Crystal" @default.
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• W1243823141 doi "https://doi.org/10.1103/physrevlett.115.083902" @default.
• W1243823141 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/26340190" @default.
• W1243823141 hasPublicationYear "2015" @default.
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