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• W128396816 abstract "Over wide ranges in temperature and time scale the stress-strain behavior of amorphous gum elastomers, up to and including break, is simply and directly related to the molecular architecture. Since rubbery behavior requires a chain-like molecular structure, the architecture of such materials on a molecular scale must be essentially similar. Differences in chain construction, e.g. in the number of chains per unit volume, should therefore give rise to specific differences in the mechanical behavior which are, even at rupture, independent of the chemical nature of the material. This essential similarity in behavior has been confirmed and so it is now possible to establish failure criteria for both uni- and multi-axial conditions which are based only on molecular parameters. The addition of a filler changes the mechanical behavior in several ways. One of the most thoroughly investigated changes is that in the small-strain modulus as a function of filler content, culminating in the theories of van der Poel, Hashin and Prager. From the first of these theories there may be obtained explicit expression for relative modulus; from the latter two, an upper and lower bound. At higher strains the rubber tends to rupture internally. At increasing strains the void usually advances to the surface of the particle and the rubber pulls away from the surface in a dewetting phenomenon. At very high loadings, or with particles which interact strongly with each other, it may be necessary to consider the contribution of particle-particle interaction forces to the overall behavior. In spite of these complications introduced by the filler, many of the characteristics of the fracture behavior of pure rubbers persist in the two-phase system, often to such an extent that the same or very similar correlative procedures may be employed. For example, time—temperature superposition is often obeyed, the rupture properties are a direct function of the number of molecular chains per unit volume of the rubber phase, and the Smith failure envelope criteria for uniaxial rupture is usually applicable. On the other hand, the presence of the filler also provides an upper bound to a strain failure criterion, since lateral contractions are possible only up to the maximum packing density of the particles." @default.
• W128396816 created "2016-06-24" @default.
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• W128396816 date "1967-01-01" @default.
• W128396816 modified "2023-10-16" @default.
• W128396816 title "SOME EFFECTS OF FILLERS ON THE DEFORMATION AND RUPTURE OF AN ELASTOMER**This paper constitutes one phase of research performed by the Jet Propulsion Laboratory, California Institute of Technology, sponsored by the National Aeronautics and Space Administration, Contract NAS7-100." @default.
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• W128396816 doi "https://doi.org/10.1016/b978-1-4831-9837-8.50029-6" @default.
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