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• W134193303 abstract "In spite of intensive experimental and theoretical studies, no model at the atomic scale has been proposed to explain the large piezoelectric effect in ${text{PbZr}}_{0.52}{text{Ti}}_{0.48}{text{O}}_{3}$ (PZT) compared to the low piezoelectric response in the simple end-member lead titanate ${text{PbTiO}}_{3}$. X-ray absorption spectroscopy (XAS) appears as the technique of choice not only to clarify the role of Zr, but also to quantify the Zr displacement through the Ferroelectric-Paraelectric $(Ftext{ensuremath{-}}P)$ transition. We clearly show evidence of the polar character of the Zr-atoms in PZT with a Zr-shift which will produce a small polarization. Such an atomic configuration for one type of atoms leads to relatively easy switching, i.e., relatively low electric field to align the Zr-polar atoms, which will create a favorable energetic situation for the cooperative switching of the strongly polar Ti-O dipole and would therefore account for the large piezoelectric effect in PZT." @default.
• W134193303 created "2016-06-24" @default.
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• W134193303 date "2010-05-12" @default.
• W134193303 modified "2023-10-14" @default.
• W134193303 title "Zr-shift at the origin of the exceptional piezoelectric properties of<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mtext>PbZr</mml:mtext></mml:mrow><mml:mrow><mml:mn>0.52</mml:mn></mml:mrow></mml:msub><mml:msub><mml:mrow><mml:mtext>Ti</mml:mtext></mml:mrow><mml:mrow><mml:mn>0.48</mml:mn></mml:mrow></mml:msub><mml:msub><mml:mtext>O</mml:mtext><mml:mn>3</mml:mn></mml:msub></mml:mrow></mml:math>" @default.
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• W134193303 doi "https://doi.org/10.1103/physrevb.81.174110" @default.
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