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- W14081442 abstract "We report the development of new experimental capabilities and ab initio modeling for real-time studies of Li-ion battery electrochemical reactions. We developed three capabilities for in-situ transmission electron microscopy (TEM) studies: a capability that uses a nanomanipulator inside the TEM to assemble electrochemical cells with ionic liquid or solid state electrolytes, a capability that uses on-chip assembly of battery components on to TEM-compatible multi-electrode arrays, and a capability that uses a TEM-compatible sealed electrochemical cell that we developed for performing in-situ TEM using volatile battery electrolytes. These capabilities were used to understand lithiation mechanisms in nanoscale battery materials, including SnO{sub 2}, Si, Ge, Al, ZnO, and MnO{sub 2}. The modeling approaches used ab initio molecular dynamics to understand early stages of ethylene carbonate reduction on lithiated-graphite and lithium surfaces and constrained density functional theory to understand ethylene carbonate reduction on passivated electrode surfaces." @default.
- W14081442 created "2016-06-24" @default.
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- W14081442 date "2012-01-01" @default.
- W14081442 modified "2023-09-27" @default.
- W14081442 title "Real-time studies of battery electrochemical reactions inside a transmission electron microscope." @default.
- W14081442 doi "https://doi.org/10.2172/1038174" @default.
- W14081442 hasPublicationYear "2012" @default.
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