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- W1427301504 abstract "In this paper, a systematic investigation on the behavior of emulsions stabilized by the mixture of hydroxyapatite (HA) nanoparticles and sodium oleate was conducted. Surprisingly, in addition to the observation of double inversion of emulsion, antagonistic effect was first discovered in surfactant range of forming W/O emulsion, in which the emulsion breaks rapidly and completely as both particles and surfactants lose their ability to stabilize oil/water interface. The origin is attributed to the adsorption of nearly all surfactant molecules on particle surfaces and the consequent transfer of sufficient hydrophobic particles from water phase into oil phase, and the surfactant molecules left are too few to stabilize oil/water interface. In this process, the oil/water interface facilitates particles’ transferring into oil phase through peeling off the second layer of surfactant because of the competition adsorption between oil/water interface and the saturated surface of HA nanoparticles. The deduction above is well supported by the results of TEM, XRD, contact angle, surface tension, TG and FTIR. This novel finding not only offers deeper recognition about roles of both HA particles and surfactant at the oil/water interfaces but also clarifies specific requirements of antagonistic effect of emulsion, which help avoiding its negative impact on the fabrication of targeting materials of HA for specific applications or enhancing the phase transfer of HA nanoparticles from water to oil for stable dispersion in oil phase." @default.
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- W1427301504 date "2015-11-01" @default.
- W1427301504 modified "2023-10-16" @default.
- W1427301504 title "Antagonistic effect in pickering emulsion stabilized by mixtures of hydroxyapatite nanoparticles and sodium oleate" @default.
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- W1427301504 doi "https://doi.org/10.1016/j.colsurfa.2015.08.009" @default.
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