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• W1428772616 abstract "This chapter discusses the use of the fluorescence of adsorbed dyes to explore the competition among the processes, which determine Φi. The basic strategy relies on measuring either τf or Φf when injection is blocked and when it is not, while assuming that ka is the same in both cases. Fluorescence quantum yields can, at least in principle, provide the same information as fluorescence lifetimes, as long as kf may also be assumed not to depend on the surface. However, if the dye is adsorbed at more than one type of surface site, only a weighted average of Φf is obtained. By contrast, time-resolved fluorescence measurements can provide both the lifetimes and the relative contributions of more than one adsorption site, and thus afford a much less encumbered look at the decay of D*. Unfortunately, while it is relatively easy to resolve contributions of widely different lifetimes, those with close lifetimes cannot be readily separated. The severity of this limitation depends on the quality of the data and on whether decay functions other than exponential have to be explored. The results surveyed in this chapter raise several important questions and suggest future experiments, which may help answer them." @default.
• W1428772616 created "2016-06-24" @default.
• W1428772616 creator A5041151594 @default.
• W1428772616 date "1989-01-01" @default.
• W1428772616 modified "2023-09-25" @default.
• W1428772616 title "Fluorescence of Dye Molecules Adsorbed on Semiconductor Surfaces" @default.
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• W1428772616 doi "https://doi.org/10.1016/s0167-2991(08)61203-3" @default.
• W1428772616 hasPublicationYear "1989" @default.
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