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- W14600615 abstract "This project has received DOE support since July 1, 1978. During this period, 40 papers have been published dealing predominantly with chlorophyll-photosensitized electron transfer reactions in a variety of media (solutions, polymer films, lipid bilayer membranes). The overall theme of this work has been to develop mechanistic strategies f or photochemical energy storage via chlorophyll, using the green plant photosynthetic system as a paradigm for designing in vitro systems. Microheterogeneous lipid vesicle suspensions allow ready application of time-resolved optical spectroscopy to follow the course of light-induced electron transfer processes. Both the yields and the lifetimes of electron transfer products were markedly improved in the vesicle systems. In subsequent studies, this compartmentalization was favorably manipulated by controlling the electrical charge on the membrane surface, by controlling the solubility properties of the acceptors, by varying the lipid composition, by using mediators to create a concentration gradient to carry electrons from within the bilayer to the aqueous medium, and by incorporating secondary electron acceptors into the aqueous phase." @default.
- W14600615 created "2016-06-24" @default.
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- W14600615 date "1994-06-16" @default.
- W14600615 modified "2023-10-03" @default.
- W14600615 title "Photochemical energy conversion by membrane-bound photoredox systems. Final report" @default.
- W14600615 doi "https://doi.org/10.2172/10106148" @default.
- W14600615 hasPublicationYear "1994" @default.
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