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• W1471202212 abstract "Kinetic and equilibrium uptake studies of selenite in aqueous solution with synthetic magnetite (Mag-P), commercial magnetite (Mag-C), goethite, activated carbon (AC), and a composite material containing 19% magnetite supported on activated carbon (CM-19) were investigated. Kinetic uptake studies used a one-pot setup at pH 5.26 at variable temperature. Sampling of unbound selenite in-situ was achieved with analytical detection by atomic absorbance. The sorptive uptake at equilibrium and kinetic conditions are listed in descending order: goethite>Mag-P>Mag-C>CM-19. Kinetic uptake parameters reveal that Mag-P showed apparent negative values for the activation energy (E(a)) and the enthalpy of activation (ΔH(‡)), in agreement with a multi-step process for the kinetic uptake of selenite. By contrast, Mag-C, CM-19, and goethite showed positive values for E(a) and ΔH(‡). The uptake properties of the various sorbent materials with selenite are in accordance with the formation of inner- and out-sphere complexes. Leaching of iron from the composite material (CM-19) was attenuated due to the stabilizing effect of the magnetite within the pore sites and the surface of AC. Supported iron oxide nanomaterial composites represent a unique sorbent material with tunable uptake properties toward inorganic selenite in aqueous solution." @default.
• W1471202212 created "2016-06-24" @default.
• W1471202212 creator A5005237155 @default.
• W1471202212 creator A5027448917 @default.
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• W1471202212 date "2015-11-01" @default.
• W1471202212 modified "2023-10-16" @default.
• W1471202212 title "Sorptive uptake of selenium with magnetite and its supported materials onto activated carbon" @default.
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• W1471202212 doi "https://doi.org/10.1016/j.jcis.2015.07.013" @default.
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