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• W1480526073 abstract "Vacancy and antisite defect formation energies in B82–SnTi2 are calculated by an ab initio approach. Three sublattices are introduced to account for the B82 structure. A statistical model based on a mean-field approximation is developed in the canonical ensemble. The defect concentrations are calculated as function of temperature and deviation from stoichiometry. For stoichiometric B82–SnTi2 alloys, the dominant thermal defects are composed of one antisite Ti atom and three Ti vacancies. In the Sn-rich B82–SnTi2, the constitutional defects are Ti vacancies; the thermal defect below 1000 K is an interbranch where Ti vacancies are replaced by Sn antisites; at high temperatures, it is a four point-defect comprising one Ti antisite and three Ti vacancies. In the Ti-rich B82–SnTi2, the constitutional defects are antisite Ti atoms and the thermal defect is a four point defect comprising one Ti antisite and three Ti vacancies. The effective defect formation enthalpies are derived at low temperature. The Gibbs energy as well as the Sn and Ti chemical potentials in B82–SnTi2 phase are obtained as function of composition for various temperatures. The extension of the one-phase domain of B82–SnTi2 in the Sn–Ti phase diagram is discussed." @default.
• W1480526073 created "2016-06-24" @default.
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• W1480526073 date "2009-05-01" @default.
• W1480526073 modified "2023-10-18" @default.
• W1480526073 title "Constitutional and thermal defects in B82–SnTi2" @default.
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• W1480526073 doi "https://doi.org/10.1016/j.intermet.2008.11.014" @default.
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