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- W1482207949 abstract "Abstract : The galvanostatic double charging method was applied to determine the coverage of Ni cathodes with adsorbed atomic H in 2 N NaOH solutions. Anodic current densities were varied from 0.05 to 1.8 amp/sq cm. The plateau indicating absence of readsorption was between 0.6 and 1.8 amp/sq cm, for a constant cathodic c.d. of 1/10,000 amp/sq cm. The variation of the adsorbed H over cathodic c.d.'s ranging from 10 to the -6th power to 1/10 at a constant anodic c.d. of 1 amp/sq cm were calculated and the coverage calculated. The mechanism of the H evolution reaction was elucidated. The rate determining step is discharge from a water molecules followed by rapid Tafel recombination. The rate constants for these processes and the rate constant for the ionisation, calculated with the extrapolated value of coverage for the reversible H electrode, were determined. A modification of the Tafel equation which takes into account both coverage and ionisation is in harmony with the results. A new method for the determination of coverage suitable for corrodible metals is described which involves the measurement of the rate of permeation of H by electrochemical techniques which enhances the sensitivity of the method." @default.
- W1482207949 created "2016-06-24" @default.
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- W1482207949 date "1961-02-28" @default.
- W1482207949 modified "2023-09-27" @default.
- W1482207949 title "THE DETERMINATION OF THE COVERAGE ON NICKEL AND STEEL DURING ELECTROLYTIC HYDROGEN EVOLUTION" @default.
- W1482207949 doi "https://doi.org/10.21236/ad0254474" @default.
- W1482207949 hasPublicationYear "1961" @default.
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