FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W1482493364> ?p ?o ?g. }

• W1482493364 endingPage "3342" @default.
• W1482493364 startingPage "3328" @default.
• W1482493364 abstract "We investigate issues related to volatility and multi‐generational gas‐phase aging parameterizations affecting the formation and evolution of secondary organic aerosol (SOA) in models. We show that when assuming realistic values for the mass accommodation coefficient, experimentally observed SOA evaporation rates imply significantly lower “effective volatility” than those derived from SOA growth in smog chambers, pointing to the role of condensed phase processes and suggesting that models need to use different parameters to describe the formation and evolution of SOA. We develop a new, experimentally driven paradigm to represent SOA as a non‐absorbing semi‐solid with very low “effective volatility.” We modify both a box model and a 3D chemical transport model, to include simplified parameterizations capturing the first‐order effects of gas‐phase fragmentation reactions and investigate the implications of treating SOA as a non‐volatile, non‐absorbing semi‐solid (NVSOA). Box model simulations predict SOA loadings decrease with increasing fragmentation, and similar SOA loadings are calculated in the traditional, semi‐volatile (SVSOA) approach and with the new paradigm (NVSOA) before evaporation reduces loadings of SVSOA. Box‐model‐calculated O:C ratios increase with aging in both the SVSOA and the NVSOA paradigms. Consistent with box model results, 3D model simulations demonstrate that predicted SOA loadings decrease with the addition of fragmentation reactions. The NVSOA paradigm predicts higher SOA loadings compared to the SVSOA paradigm over nearly the entire 3D modeling domain, with larger differences close to the surface and in regions where higher dilution favors SVSOA evaporation." @default.
• W1482493364 created "2016-06-24" @default.
• W1482493364 creator A5009113528 @default.
• W1482493364 creator A5015242085 @default.
• W1482493364 creator A5040702506 @default.
• W1482493364 creator A5047588154 @default.
• W1482493364 creator A5056263999 @default.
• W1482493364 creator A5074206807 @default.
• W1482493364 creator A5091599490 @default.
• W1482493364 date "2013-04-16" @default.
• W1482493364 modified "2023-10-10" @default.
• W1482493364 title "Implications of low volatility SOA and gas-phase fragmentation reactions on SOA loadings and their spatial and temporal evolution in the atmosphere" @default.
• W1482493364 cites W1561878391 @default.
• W1482493364 cites W1968862760 @default.
• W1482493364 cites W1969061516 @default.
• W1482493364 cites W1970419627 @default.
• W1482493364 cites W1973477740 @default.
• W1482493364 cites W1982056270 @default.
• W1482493364 cites W1985285121 @default.
• W1482493364 cites W1986418366 @default.
• W1482493364 cites W1990687171 @default.
• W1482493364 cites W1994506621 @default.
• W1482493364 cites W2005556999 @default.
• W1482493364 cites W2010619046 @default.
• W1482493364 cites W2013766417 @default.
• W1482493364 cites W2015133270 @default.
• W1482493364 cites W2023037439 @default.
• W1482493364 cites W2029337195 @default.
• W1482493364 cites W2031457789 @default.
• W1482493364 cites W2039437298 @default.
• W1482493364 cites W2042175812 @default.
• W1482493364 cites W2047926788 @default.
• W1482493364 cites W2050868506 @default.
• W1482493364 cites W2051730874 @default.
• W1482493364 cites W2052859509 @default.
• W1482493364 cites W2054552851 @default.
• W1482493364 cites W2059510438 @default.
• W1482493364 cites W2067318157 @default.
• W1482493364 cites W2078555613 @default.
• W1482493364 cites W2081922930 @default.
• W1482493364 cites W2098012332 @default.
• W1482493364 cites W2099917135 @default.
• W1482493364 cites W2102708663 @default.
• W1482493364 cites W2106115411 @default.
• W1482493364 cites W2109419617 @default.
• W1482493364 cites W2115381341 @default.
• W1482493364 cites W2116507044 @default.
• W1482493364 cites W2116608634 @default.
• W1482493364 cites W2122530338 @default.
• W1482493364 cites W2122770087 @default.
• W1482493364 cites W2123971863 @default.
• W1482493364 cites W2133032938 @default.
• W1482493364 cites W2134662674 @default.
• W1482493364 cites W2144188667 @default.
• W1482493364 cites W2144923407 @default.
• W1482493364 cites W2145220145 @default.
• W1482493364 cites W2153555750 @default.
• W1482493364 cites W2161164864 @default.
• W1482493364 cites W2163144959 @default.
• W1482493364 cites W2163510770 @default.
• W1482493364 cites W2166349750 @default.
• W1482493364 cites W2170783614 @default.
• W1482493364 cites W2171810356 @default.
• W1482493364 cites W2172118306 @default.
• W1482493364 cites W2323117465 @default.
• W1482493364 cites W2334088731 @default.
• W1482493364 doi "https://doi.org/10.1002/jgrd.50160" @default.
• W1482493364 hasPublicationYear "2013" @default.
• W1482493364 type Work @default.
• W1482493364 sameAs 1482493364 @default.
• W1482493364 citedByCount "67" @default.
• W1482493364 countsByYear W14824933642014 @default.
• W1482493364 countsByYear W14824933642015 @default.
• W1482493364 countsByYear W14824933642016 @default.
• W1482493364 countsByYear W14824933642017 @default.
• W1482493364 countsByYear W14824933642018 @default.
• W1482493364 countsByYear W14824933642019 @default.
• W1482493364 countsByYear W14824933642020 @default.
• W1482493364 countsByYear W14824933642021 @default.
• W1482493364 countsByYear W14824933642022 @default.
• W1482493364 countsByYear W14824933642023 @default.
• W1482493364 crossrefType "journal-article" @default.
• W1482493364 hasAuthorship W1482493364A5009113528 @default.
• W1482493364 hasAuthorship W1482493364A5015242085 @default.
• W1482493364 hasAuthorship W1482493364A5040702506 @default.
• W1482493364 hasAuthorship W1482493364A5047588154 @default.
• W1482493364 hasAuthorship W1482493364A5056263999 @default.
• W1482493364 hasAuthorship W1482493364A5074206807 @default.
• W1482493364 hasAuthorship W1482493364A5091599490 @default.
• W1482493364 hasBestOaLocation W14824933642 @default.
• W1482493364 hasConcept C111919701 @default.
• W1482493364 hasConcept C121332964 @default.
• W1482493364 hasConcept C149782125 @default.
• W1482493364 hasConcept C153294291 @default.
• W1482493364 hasConcept C191015642 @default.
• W1482493364 hasConcept C192562407 @default.
• W1482493364 hasConcept C2779345167 @default.
• W1482493364 hasConcept C33923547 @default.

• next