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- W1483441610 abstract "The activity and selectivity of the alumina-supported molybdenum carbide for the HDN ofcarbazole were studied. The effects of catalyst pretreatment and surface composition of the supported Mo carbides on the HDN activity of the catalyst were also considered. Catalyst characterization was done using TPR, BET, nitrogen element, XRD, and XPS analyses. It was revealed that the catalyst carburized at 700°C was 2.2 times more active than was the catalyst carburized at 500°C in the HDN of carbazole. The TPR analysis showed that neither transformation of the Mo nitrides to the Mo carbides nor free-carbon deposition occurs below 500°C for the alumina-supported catalysts, although above 900°C, a large amount of free carbon is deposited on the surface of the Mo carbide catalysts. For the unsupported Mo catalysts, the XRD analysis showed that Mo2N was converted to α-Mo2C at 700°C, and above 900°C the α-Mo2C crystal was transformed to η-Mo3C2 crystal." @default.
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- W1483441610 date "1997-01-01" @default.
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- W1483441610 title "Surface property of alumina-supported Mo carbide and its activity for HDN" @default.
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- W1483441610 doi "https://doi.org/10.1016/s0167-2991(97)80022-5" @default.
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