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- W1483610062 abstract "We describe a Brillouin spectroscopy system integrated with CO2 laser-heating and Raman spectroscopic capabilities. Temperature is determined by measurements of the grey-body thermal radiation emitted by the hot sample, with the system response calibrated relative to a standard tungsten ribbon lamp. High-pressure laser-heating Brillouin scattering measurements of acoustic velocities on liquid water and ice compressed in a diamond-anvil cell were performed at temperatures up to 2500 ± 150 K at high pressure. Single-crystal laser-heating Brillouin measurements were made on the (111) plane of San Carlos olivine at ∼13 GPa, 1300 ± 200 K. The pressure as measured by ruby fluorescence is shown to be within ±0.5 GPa of the pressure on the olivine sample during laser heating when KCl and KBr are used as pressure-transmitting media. In addition, the system is designed for continuously variable scattering angles from forward scattering (near 0° scattering angle) up to near back scattering (∼141°). This novel setup allows us to probe a wide range of wave vectors q for investigation of phonon dispersion on, for example, crystals with large unit cells (on the scale of hundreds of nm)." @default.
- W1483610062 created "2016-06-24" @default.
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- W1483610062 date "2015-06-01" @default.
- W1483610062 modified "2023-10-13" @default.
- W1483610062 title "Single-crystal Brillouin spectroscopy with CO2 laser heating and variable q" @default.
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- W1483610062 doi "https://doi.org/10.1063/1.4922634" @default.
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