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• W1489366842 abstract "Experimental measurements clearly reveal the presence of bulk superconductivity in the CsPbxBi4−xTe6 (0.3≤x≤1.0) materials, i.e. the first member of the thermoelectric series of Cs[PbmBi3Te5+m], these materials have the layered orthorhombic structure containing infinite anionic [PbBi3Te6]− slabs separated with Cs+ cations. Temperature dependences of electrical resistivity, magnetic susceptibility, and specific heat have consistently demonstrated that the superconducting transition in Cs0.96Pb0.25Bi3.75Te6.04 occurs at Tc=3.1 K, with a superconducting volume fraction close to 100% at 1.8 K. Structural study using aberration-corrected STEM/TEM reveals a rich variety of microstructural phenomena in correlation with the Pb-ordering and chemical inhomogeneity. The superconducting material Cs0.96Pb0.25Bi3.75Te6.04 with the highest Tc shows a clear ordered structure with a modulation wave vector of q≈a*/2+c*/1.35 on the a–c plane. Our study evidently demonstrates that superconductivity deriving upon doping of narrow-gap semiconductor is a viable approach for exploration of novel superconductors." @default.
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• W1489366842 date "2015-12-01" @default.
• W1489366842 modified "2023-10-15" @default.
• W1489366842 title "Superconductivity in the orthorhombic phase of thermoelectric CsPbxBi4−xTe6 with 0.3≤x≤1.0" @default.
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• W1489366842 doi "https://doi.org/10.1016/j.jssc.2015.08.050" @default.
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