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- W1489388210 abstract "Introduction The unique ability of silver to selectively catalyze the partial oxidation of ethylene to ethylene oxide has attracted scientific interest in this system for several decades. Although the selectivity of this reaction in industrial processes has exceeded 80 %, research is still continuing in the field since there is no thermodynamic limit for further increasing selectivity. Recently Barteau et al. found that copper-silver bimetallic catalysts offer improved selectivities compared to pure silver in the direct epoxidation of ethylene [1]. Due to the low adsorption enthalpy, ethylene epoxidation is impossible to study under UHV conditions. This limits the information regarding the chemical state of the surface and adsorbents under reaction conditions. Thus many fundamental questions concerning the mechanism of the reaction remain controversial. Recent development of a photoelectron spectroscopy apparatus, which is able to operate in the mbar pressure range, allows monitoring of the chemical status of the surface under working catalytic conditions." @default.
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- W1489388210 date "2007-01-01" @default.
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- W1489388210 title "Ethylene epoxidation over copper-silver bimetallic catalyst: surface characterisation under reaction conditions" @default.
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