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- W1489626114 abstract "The cubic AuCu‐type intermetallic compounds AnRh3 (where An=Th, U, Np and Pu) have been prefiously studied and were found to exhibit 5f electron character similar to pur actinide metals; i.e., no 5f band in ThRh3 and a broad hybridized 5f‐6d band in URh3 which becomes progressively narrower as the actinide component is substituted across the actinide series. The purpose of the present investigation is to determine the U concentration x in the UxTH1−xRh3 system which first manifests evidence for an occupied hybridized 5f–6d band. The room‐temperature magnetic susceptibilities, electrical resistivities, and lattice parameters were measured for x=0, 0.1, 0.3, 0.5, 0.7, 0.9 and 1.0. A sharp break in the plot of room temperature parameters vs x is observed at x‐ 0.4 for susceptibility and x‐ 0.55 for resistivity with both parameters increasing much more rapidly at higher values of x. The sharp rise is attributed to the introduction of an electron band with a high density of states at the Fermi level. It is believed that this is a hybridized 5f‐6d band. The discrepancy between the resistivity and susceptibility results is not understood, but magnetic susceptibility is judged to be more closely related to the density of states and hence a better indicator of the introduction of 5f electrons." @default.
- W1489626114 created "2016-06-24" @default.
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- W1489626114 date "1975-01-01" @default.
- W1489626114 modified "2023-09-24" @default.
- W1489626114 title "The onset of the 5f energy band in Th1−xUxRh3 intermetallic compounds" @default.
- W1489626114 doi "https://doi.org/10.1063/1.30133" @default.
- W1489626114 hasPublicationYear "1975" @default.
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