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- W1489885871 abstract "We report magneto-photoluminescence studies of strongly quantum-confined 0-D diluted magnetic semiconductors (DMS), realized in Mn$^{2+}$-doped ZnSe/CdSe core/shell colloidal nanocrystals. In marked contrast to their 3-D (bulk), 2-D (quantum well), 1-D (quantum wire), and 0-D (self-assembled quantum dot) DMS counterparts, the ubiquitous yellow emission band from internal emph{d-d} ($^4T_1 rightarrow ^6A_1$) transitions of the Mn$^{2+}$ ions in these nanocrystals is emph{not} suppressed in applied magnetic fields and emph{does} become circularly polarized. This polarization tracks the Mn$^{2+}$ magnetization, and is accompanied by a sizable energy splitting between right- and left-circular emission components that scales with the exciton-Mn emph{sp-d} coupling strength (which, in turn, is tunable with nanocrystal size). These data highlight the influence of strong quantum confinement on both the excitation and the emission mechanisms of magnetic ions in DMS nano-materials." @default.
- W1489885871 created "2016-06-24" @default.
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- W1489885871 date "2011-08-03" @default.
- W1489885871 modified "2023-09-30" @default.
- W1489885871 title "Spin-Polarized<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:msup><mml:mi>Mn</mml:mi><mml:mrow><mml:mn>2</mml:mn><mml:mo>+</mml:mo></mml:mrow></mml:msup></mml:math>Emission from Mn-Doped Colloidal Nanocrystals" @default.
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- W1489885871 doi "https://doi.org/10.1103/physrevlett.107.067402" @default.
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