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- W1495104080 abstract "It has been prepared Nb-ilerite and Me/Nb-ilerite (Me = Pt, Pd) catalysts with pillaring and impregnation methods using the layered silicate of ilerite structure as a host material, and carried out vapor phase Beckmann rearrangement of cyclohexanone oxime to ε-caprolactam for the catalysts. It was found that Pt and Pd metals played very important role to improve the catalytic performance of Nb-ilerite. Pt/Nb-ilerite and Pd/Nb-ilerite catalysts exhibited higher lactam selectivities and yields than Nb-ilerite catalyst. Particularly, Pt//Nb-ilerite showed a relatively strong resistance for catalyst deactivation. NH3-TPD measurements for the catalysts revealed that these results were mainly due to the change of acidic properties of the catalysts by metal loading." @default.
- W1495104080 created "2016-06-24" @default.
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- W1495104080 date "2004-01-01" @default.
- W1495104080 modified "2023-09-25" @default.
- W1495104080 title "Vapor phase Beckmann rearrangement of cyclohexanone oxime over metal loaded Nb-ilerite" @default.
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- W1495104080 doi "https://doi.org/10.1016/s0167-2991(04)80559-7" @default.
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