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- W1497182942 abstract "A novel photochemical method of removing reactive fluorides from UF{sub 6} gas has been discovered. This method reduces generated waste to little more than the volume of the removed impurities, minimizes loss of UF{sub 6}, and can produce a recyclable by-product, fluorine gas. In our new method, impure UF{sub 6}, is exposed to ultraviolet light which dissociates the UF{sub 6} to UF{sub 5} and fluorine atom. Impurities which chemically react with UF{sub 5} are reduced and form solid compounds easily removed from the gas while UF{sub 5} is converted back to UF{sub 6}. Proof-of-concept testing involved UF{sub 6} containing NpF{sub 6} and PuF{sub 6} with CO added as a fluorine atom scavenger. In a single photolysis step, greater than 5000-fold reduction of PuF{sub 6} was demonstrated while reducing NpF{sub 6} by more than 40-fold. This process is likely to remove corrosion and fission product fluorides that are more reactive than UF{sub 6} and has been demonstrated without an added fluorine atom scavenger by periodically removing photogenerated fluorine gas. 44 refs., 3 figs., 2 tabs." @default.
- W1497182942 created "2016-06-24" @default.
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- W1497182942 date "1990-01-01" @default.
- W1497182942 modified "2023-09-24" @default.
- W1497182942 title "Photochemical removal of NpF sub 6 and PuF sub 6 from UF sub 6 gas streams" @default.
- W1497182942 hasPublicationYear "1990" @default.
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