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- W1497334841 abstract "Non-resonant inelastic x ray scattering (NIXS) experiments have been performed to probe the 5d-5f electronic transitions at the uranium O(4,5) absorption edges in uranium dioxide. For small values of the scattering vector q, the spectra are dominated by dipole-allowed transitions encapsulated within the giant resonance, whereas for higher values of q the multipolar transitions of rank 3 and 5 give rise to strong and well-defined multiplet structure in the pre-edge region. The origin of the observed non-dipole multiplet structures is explained on the basis of many-electron atomic spectral calculations. The results obtained demonstrate the high potential of NIXS as a bulk-sensitive technique for the characterization of the electronic properties of actinide materials." @default.
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- W1497334841 date "2010-05-05" @default.
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- W1497334841 title "Uranium<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mn>5</mml:mn><mml:mi>d</mml:mi><mml:mtext>−</mml:mtext><mml:mn>5</mml:mn><mml:mi>f</mml:mi></mml:mrow></mml:math>electric-multipole transitions probed by nonresonant inelastic x-ray scattering" @default.
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- W1497334841 doi "https://doi.org/10.1103/physrevb.81.195104" @default.
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