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- W1499777640 abstract "ABSTRACT The kinetics of the CO + NO reactions has been studied at 300 °C over a fresh and a deactivated bimetallic Pt-Rh/Al 2 O 3 catalyst. Two kinetic models have been examined including competitive and non-competitive adsorptions of the reactants. The discrimination between these two assumptions has been achieved by using graphic and mathematical methods. From the comparison of kinetic and thermodynamic constants calculated from these methods with those previously obtained on Rh/Al 2 O 3 and on Pt/Al 2 O 3 , we believe that the kinetic data obtained on the fresh Pt-Rh/Al 2 O 3 catalyst can be modelled by non-competitive adsorptions of the reactants assuming a preferential adsorption of NO on Rh and CO on Pt. By contrast NO and CO competitive adsorptions can only occur on the deactivated Pt-Rh/Al 2 O 3 catalyst, which to assume that the active surface is mostly composed of Rh." @default.
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- W1499777640 date "1998-01-01" @default.
- W1499777640 modified "2023-09-25" @default.
- W1499777640 title "Investigation on the role of Rhodium on the kinetics of the oxidation of CO by NO over Pt-Rh catalysts" @default.
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- W1499777640 doi "https://doi.org/10.1016/s0167-2991(98)80898-7" @default.
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