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- W1504057100 abstract "ENDOR measurements have been made on 19F ligand, 23Na and second-neighbour 19F nuclei surrounding the dilute paramagnetic sites in single crystals of K2NaAlF6:Fe3+, Cr3+. On the basis that the main contribution to the isotropic transferred hyperfine interactions with the 23Na and second-neighbour 19F nuclei is through overlap mechanisms with the ligand 2p orbitals, the data have been interpreted by comparison of the relative values of these quantities in the two systems. The result is that the unpaired spin fractions for the ligand 2p orbitals, fsigma and fpi , may be estimated independently and are found to be in general agreement with other methods, particularly in the verification of a significant negative fsigma for the (CeF6)3- complex. Little evidence of ligand polarisation is found in these systems." @default.
- W1504057100 created "2016-06-24" @default.
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- W1504057100 date "1981-02-20" @default.
- W1504057100 modified "2023-10-18" @default.
- W1504057100 title "ENDOR determination of covalency in K2NaAlF6:Fe3+, Cr3+" @default.
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- W1504057100 doi "https://doi.org/10.1088/0022-3719/14/5/003" @default.
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