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• W1504724075 startingPage "357" @default.
• W1504724075 abstract "Publisher Summary It is recognized that the surfaces of oxides are geometrically distorted and therefore energetically heterogeneous for adsorption. It has been realized by the scientists investigating adsorption from the gas phase for a long time. Dozens of papers were published showing that successful correlations of the experimental data for gas adsorption onto oxides can be done only by using equations corresponding to a heterogeneous surface model. The experimental studies were stimulated strongly by the widely spread view that these are the surface imperfections creating catalytic centers for many important catalytic reactions. Bakaev's computer simulations of oxide surfaces suggest that even in the case of oxides having a well defined bulk crystal structure, the degree of the surface disorder may be larger than it is generally believed. The chapter focuses its attention on the extremely important class of adsorption systems, composed of water being in contact with oxide surfaces. The reasons, why the behavior of water/oxide interfaces is so important for various areas of science, life, and industry, are well-known. The chapter analyzes a variety of adsorption data obtained while investigating the adsorption at oxide/water vapor interface, and oxide/electrolyte interface. That analysis summarized the extensive research conducted during the past few years, and concerning the model of adsorption on oxide surfaces. The analysis shows, that only the model of energetically heterogeneous surface can be a proper basis for a successful theoretical description of adsorption at water vapor/oxide, and oxide/electrolyte interfaces. It is also demonstrated, that a simultaneous analysis of adsorption isotherms and heats of adsorption may lead to a new level of understanding the mechanism of adsorption in those systems." @default.
• W1504724075 created "2016-06-24" @default.
• W1504724075 creator A5014842582 @default.
• W1504724075 creator A5041874660 @default.
• W1504724075 creator A5069799552 @default.
• W1504724075 date "1996-01-01" @default.
• W1504724075 modified "2023-10-03" @default.
• W1504724075 title "Chapter 2.2 On the nature of the energetic heterogeneity of water/oxide interface in adsorption phenomena occurring at oxide surfaces" @default.
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