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- W1505280557 abstract "Parallel optical and electrochemical studies on the V(III)/V(II) system in H2O + acetonitrile (AN) + CF3SO3H mixtures have been performed. It was found, on the basis of the spectra of vanadium ions in the visible range, that V(III) was totally hydrated in mixtures up to xAN ⋍ 0.6 while V(II) was specifically solvated by AN molecules, even at a molar fraction of acetonitrile in H2O + AN mixtures as low as 0.02. In agreement with this, the formal potentials of the V(III)/V(II) system expressed versus the ferrocene electrode move to less negative potentials with an increase in AN concentration. Straightforward correlations of the electrode kinetics of the V(III)/V(II) system at a mercury electrode in H2O + AN mixtures with both the electrode surface coverage by AN molecules and the resolvation of vanadium ions in the bulk solution were found." @default.
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- W1505280557 date "1987-11-01" @default.
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- W1505280557 title "Solvent effects on the electrode kinetics of simple redox couples" @default.
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- W1505280557 doi "https://doi.org/10.1016/0022-0728(87)85234-8" @default.
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