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- W1505644559 abstract "Percolation thresholds for solvent diffusion within hydrated model polymeric membranes are derived from dissipative particle dynamics in combination with Monte Carlo (MC) tracer diffusion calculations. The polymer backbones are composed of hydrophobic A beads to which at regular intervals Y-shaped side chains are attached. Each side chain is composed of eight A beads and contains two identical branches that are each terminated with a pendant hydrophilic C bead. Four types of side chains are considered for which the two branches (each represented as [C], [AC], [AAC], or [AAAC]) are splitting off from the 8th, 6th, 4th, or 2nd A bead, respectively. Water diffusion through the phase separated water containing pore networks is deduced from MC tracer diffusion calculations. The percolation threshold for the architectures containing the [C] and [AC] branches is at a water volume fraction of ∼0.07 and 0.08, respectively. These are much lower than those derived earlier for linear architectures of various side chain length and side chain distributions. Control of side chain architecture is thus a very interesting design parameter to decrease the percolation threshold for solvent and proton transports within flexible amphiphilic polymer membranes." @default.
- W1505644559 created "2016-06-24" @default.
- W1505644559 creator A5028249395 @default.
- W1505644559 date "2015-06-08" @default.
- W1505644559 modified "2023-09-27" @default.
- W1505644559 title "Searching for low percolation thresholds within amphiphilic polymer membranes: The effect of side chain branching" @default.
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- W1505644559 doi "https://doi.org/10.1063/1.4922156" @default.
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