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- W1505754416 abstract "Hitherto, adsorption has been traditionally used to study only the porous structure in disordered materials, while the structure of the solid phase skeleton has been probed by crystallographic methods such as x-ray diffraction. Here we show that for carbons density functional theory, suitably adapted to consider heterogeneity of the pore walls, can be reliably used to probe features of the solid structure hitherto accessibly only approximately even by crystallographic methods. We investigate a range of carbons, including commercial activated carbons, activated carbon fibres as well as coal chars prepared in our laboratory, and determine pore wall thickness distributions using argon adsorption. The results are corroborated by x-ray diffraction studies, which yield a parallelism indicator that correlates well with its counterpart determined from the adsorption-based pore wall thickness distributions. Further, characterization of progressively heated carbons using the proposed approach shows clear evidence of thickening of pore walls, confirmed by xrd." @default.
- W1505754416 created "2016-06-24" @default.
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- W1505754416 date "2007-01-01" @default.
- W1505754416 modified "2023-09-24" @default.
- W1505754416 title "Characterization of nanoporous carbons" @default.
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- W1505754416 doi "https://doi.org/10.1016/s0167-2991(07)80010-3" @default.
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