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• W1506656 abstract "Oxygen plays an important, but often poorly understood, role in many photocatalytic processes. Here, we investigate the adsorption and photon-stimulated reactions of O2 on reduced rutile TiO2(110). After adsorption at 28 K and annealing to 100 K, at least 85% of the O2 has not dissociated. Typically, less than 50% of this molecularly adsorbed O2 desorbs via hole-mediated reactions during irradiation with ultraviolet (UV) photons. However, UV irradiation dissociates ∼20−45% of the chemisorbed O2, which we propose to occur through electron attachment reactions. In addition, weakly bound (physisorbed) O2 readily reacts with chemisorbed O2 during UV irradiation. These results show that the photochemistry of oxygen on TiO2(110) is both diverse and more complicated than previously appreciated." @default.
• W1506656 created "2016-06-24" @default.
• W1506656 creator A5029632614 @default.
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• W1506656 date "2010-05-21" @default.
• W1506656 modified "2023-09-27" @default.
• W1506656 title "Photoinduced Dissociation of O₂ on Rutile TiO₂(110)" @default.
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• W1506656 doi "https://doi.org/10.1021/jz100513e" @default.
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