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- W1509218488 abstract "The redox reaction IrCl2−/3−6 is investigated with inert electrodes coated with thin films of quaternized and cross-linked polyvinylpyridine. The oxidized form of the redox couple is strongly absorbed by the film, generating a “low permeability” (LP) state of the matrix characterized by a diffusion coefficient Dox ≈ 3×10−9 cm2 s−1. The presence of IrCl3−6 leads to the “high permeability” (HP) state of the membrane, in which diffusion coefficients are larger by an order of magnitude. The transition from the HP to the LP state is demonstrated. It is shown further that even in the LP state charge transport across the film proceeds predominantly by motion of the redox ions and not by electron hopping." @default.
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- W1509218488 date "1987-08-01" @default.
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- W1509218488 title "Hexachloroiridate(III/IV) on polymer-coated electrodes" @default.
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- W1509218488 doi "https://doi.org/10.1016/0022-0728(87)85142-2" @default.
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