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- W1510403216 abstract "A variable temperature-selected ion flow drift tube (VT-SIFDT) has been used to measure the mobilities of NH4+(NH3)n clusters drifting in He. The mobilities have been measured for n=0–2 at 298 K, n=0–3 at 200 K, and n=0–5 at 100 K, marking the first mobilities experiments for these clusters below room temperature. The reduced mobilities measured at 298 K are compared to the previous SIFDT results of Krishnamurthy et al. [J. Chem. Phys. 106, 530 (1997)] for n=0–2. While the current results compare quite favorably for n=0–2, there is a discrepancy for n=3 which is addressed by current 100 K and 200 K data where these species are thermally stable. The trends in the mobilities from 100 K to 298 K as a function of E/N and effective temperature reveal that the repulsive part of the He–NH4+(NH3)n interaction potential is sampled predominantly for n=1–5. However, the attractive part of the potential is accessed at the lowest temperatures for He–NH4+." @default.
- W1510403216 created "2016-06-24" @default.
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- W1510403216 date "2001-04-08" @default.
- W1510403216 modified "2023-09-25" @default.
- W1510403216 title "Mobilities of NH4+(NH3)n clusters in helium from 100 K to 298 K" @default.
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- W1510403216 doi "https://doi.org/10.1063/1.1354136" @default.
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