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- W1517764602 abstract "The droplet model of fullerene clusters in solutions is used for analysis of experimental data on the concentration dependence of the third order nonlinear optical susceptibility of fullerene C60 benzene solution and also for determination of heat of solution of fullerenes versus concentration and temperature. The absorption frequency of fullerene molecules involved into clusters is removed out the four-wave mixing resonance which causes the decrease in a number of fullerene molecules interacting with radiation. Therefore the third order nonlinear optical susceptibility is defined only by separate C60 molecules which are not involved into clusters. The use of cluster size distribution function of aggregated fullerenes in solutions found earlier provides quite good coincigence between the measured dependencies χ(1)(C) and concentration dependence of separate fullerene molecules. The same function is used for determination of the concentration and temperature dependencies of the heat of solution of aggregat..." @default.
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- W1517764602 date "1998-01-01" @default.
- W1517764602 modified "2023-09-25" @default.
- W1517764602 title "Optical properties and heat of solution of fullerenes taking account the aggregation of fullerenes in solutions" @default.
- W1517764602 doi "https://doi.org/10.1063/1.56469" @default.
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