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• W1521962406 abstract "We demonstrate the nonequilibrium tip induced control of the spin state of copper phthalocyanine on an insulator coated substrate. We find that, under the condition of energetic proximity of many-body neutral excited states to the anionic ground state, the system can undergo a population inversion towards these excited states. The resulting state of the system is accompanied by a change in the total spin quantum number. Experimental signatures of the crossover are the appearance of additional nodal planes in the topographical scanning tunneling microscopy images as well as a strong suppression of the current near the center of the molecule. The robustness of the effect against moderate charge conserving relaxation processes has also been tested." @default.
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• W1521962406 date "2016-03-16" @default.
• W1521962406 modified "2023-10-16" @default.
• W1521962406 title "Nonequilibrium spin crossover in copper phthalocyanine" @default.
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• W1521962406 doi "https://doi.org/10.1103/physrevb.93.121406" @default.
• W1521962406 hasPublicationYear "2016" @default.
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