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- W1526048589 abstract "A general procedure to simplify a complex first-order reaction by two approximations, the principle of fast equilibration and the steady-state approximation, is presented. Rate constants are classified into two groups: those of the order of unity and those of the order of ϵ(⪡ 1) or less, and are represented in the schemes by thick and thin arrows, respectively. The fast and the slow components are defined: from the fast component at least one thick arrow originates and from the slow component no thick arrow originates. Fast components are divided into several groups. In a group, the fast components are connected by thick arrows in both directions in each reaction step. When at least one thick arrow originates from the components in a group G and terminates on a component not belonging to group G (group G is open), then the steady-state approximation or principle of fast equilibration holds on each component in group G after an induction period T°. When no thick arrow originating from group G is directed to components not belonging to group G (group G is closed), the principle of fast equilibration holds on the fast components in group G after T°. The induction period T° is less than the order of I/ϵ." @default.
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- W1526048589 date "1982-11-01" @default.
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- W1526048589 title "‘Steady/equilibrium approximation’ in relaxation and fluctuation" @default.
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- W1526048589 doi "https://doi.org/10.1016/0301-4622(82)87001-4" @default.
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