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- W1526201250 abstract "Linear and cyclic ferrocenylhexasilanes 1,6-Fc-Si6Me12-X [X = Me,-C6H4CHC(CN)2], 1,3- and 1,4-Fc-Si6Me10-X [X = Me, -C6H4CHC(CN)2], have been synthesized and their Mössbauer spectra have been measured. All compounds possess localized electronic structures on the Mossbauer timescale and partial FeIIIcharacter of the iron atom due to Cp→(Sin) electron transfer. The Mossbauer data obtained, furthermore, indicate considerable aryl-ferrocenyl interaction via the hexasilane moiety. The single-crystal X-ray structures of 1,3- and 1,4-Fc-Si6Me10-C6H4CHC(CN)2 exhibit the cyclohexasilane ring in chair conformation with the bulky Fc and aryl substituents in equatorial positions, while the open-chained analogue exhibits a perfect all-trans geometry." @default.
- W1526201250 created "2016-06-24" @default.
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- W1526201250 date "2005-07-26" @default.
- W1526201250 modified "2023-10-03" @default.
- W1526201250 title "57Fe-Mössbauer Spectra and X-Ray Structures of Dipolar Ferrocenylhexasilanes" @default.
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- W1526201250 doi "https://doi.org/10.1002/9783527620777.ch75d" @default.
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