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- W1526384279 abstract "Abstract : Molecular decompositions often control complex chemical reactions by producing a highly reactive fragment that determines the subsequent chemistry. Despite the importance of such processes, there is little detailed information available for testing theoretical models and guiding the analysis of practical systems. This report describes experiments that produce, characterize, and dissociate highly energized molecules in order to uncover the details of molecular decomposition. These experiments create highly energized molecules either by vibrational overtone excitation or electronic excitation and detect the products either by a state-resolved laser detection technique, such as laser induced fluorescence, or by energy-selective ionization using vacuum ultraviolet photons. The state-resolved measurements probe the decomposition dynamics by determining the quantum state populations in the products and their appearance rates. These data provide a particularly good point of comparison with theoretical models and are a test of the applicability of statistical theories. The energy-selective ionization studies can also provide rate information but are most valuable as a means of identifying the primary dissociation products and their recoil energies. The use of vacuum ultraviolet photons makes our apparatus very sensitive. We have proven the technique on electronic photodissociation of a series of nitroalkanes and on nitrobenzene." @default.
- W1526384279 created "2016-06-24" @default.
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- W1526384279 date "1991-12-12" @default.
- W1526384279 modified "2023-09-24" @default.
- W1526384279 title "The Pathways and Dynamics of Molecular Decomposition" @default.
- W1526384279 hasPublicationYear "1991" @default.
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